Some people like Dictionaries, but I prefer Lookups due to the behavior when a key is missing.
IEnumerable<MyObj> allValues = ...
ILookup<bool, MyObj> theLookup = allValues.ToLookup(val => val.SomeProp);
// does not throw when there are not any true elements.
List<MyObj> trues = theLookup[true].ToList();
// does not throw when there are not any false elements.
List<MyObj> falses = theLookup[false].ToList();
Unfortunately, this approach enumerates twice – once to create the lookup, then once to create the lists.
If you don’t really need lists, you can get this down to a single iteration:
IEnumerable<MyObj> trues = theLookup[true];
IEnumerable<MyObj> falses = theLookup[false];